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Four-wave mixing (FWM) of optical fields has been extensively used in quantum information processing, sensing, and memories. It also forms a basis for nonlinear spectroscopies such as transient grating, stimulated Raman, and photon echo where phase matching is used to select desired components of the third-order response of matter. Here we report an experimental study of the two-dimensional quantum noise intensity difference spectra of a pair of squeezed beams generated by FWM in hot Rb vapor. The measurement reveals details of the χ ( 3 ) susceptibility dressed by the strong pump field which induces an AC Stark shift, with higher spectral resolution compared to classical measurements of probe and conjugate beam intensities. We demonstrate how quantum correlations of squeezed light can be utilized as a spectroscopic tool which unlike their classical counterparts are robust to external noise.more » « less
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Schlawin, Frank; Dorfman, Konstantin_E; Mukamel, Shaul (, The Journal of Chemical Physics)Glauber’s g(2)-function provides a common measure of quantum field statistics through two-photon coincidence counting in Hanbury Brown–Twiss measurements. Here, we propose to use nonlinear optical signals as a tool for the characterization of quantum light. In particular, we show that Raman measurements provide an alternative direct probe for a different component of the four-point correlation function underlying the g(2)-function. We illustrate this capacity for a specific quantum state obtained from a frequency conversion process. Our work points out how the analysis of controlled optical nonlinear processes can provide an alternative window toward the analysis of quantum light sources.more » « less
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Yang, Zhenquan; Saurabh, Prasoon; Schlawin, Frank; Mukamel, Shaul; Dorfman, Konstantin E. (, Applied Physics Letters)null (Ed.)
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Mukamel, Shaul; Freyberger, Matthias; Schleich, Wolfgang; Bellini, Marco; Zavatta, Alessandro; Leuchs, Gerd; Silberhorn, Christine; Boyd, Robert W; Sánchez-Soto, Luis Lorenzo; Stefanov, André; et al (, Journal of Physics B: Atomic, Molecular and Optical Physics)
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